One who is not a friend; an enemy.
It is even as I suspected, my lord, […] Ye have back-friends, my lord, that is, unfriends—or, to be plain, enemies—about the person of the Prince.
To sever as friends.
"I hope, sir, that we are not mutually Unfriended by this Difference which hath happened betwixt us."
To defriend; to remove from one's friends list (e.g. on a social networking website).
From Middle English unfreend, onfrend, equivalent to un- (noun/adjective prefix) + friend. Cognate with Scots unfrend (“unfriend”). Compare Old English unfriþmann, unwine.
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"I asked her why, she said it was because I didn't comment, and I shrugged and said whatever. I didn't unfriend her."